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RARE-EARTH AND ALKALINE-EARTH HALIDES WITH SCINTILLATION ACTIVATORS AND CO-DOPANTS STUDIED BY PICOSECOND OPTICAL ABSORPTION SPECTROSCOPY

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title
RARE-EARTH AND ALKALINE-EARTH HALIDES WITH SCINTILLATION ACTIVATORS AND CO-DOPANTS STUDIED BY PICOSECOND OPTICAL ABSORPTION SPECTROSCOPY
author
Li, Peiyun
abstract
Recent discoveries of rare-earth and alkaline-earth halides with scintillation activators and co-dopants showing excellent properties for spectroscopic gamma radiation detection attract a surge in research activity on their scintillation mechanisms. There is still much to learn about excited states in these materials. Understanding behaviors of the free carries and excitons in the first picoseconds are crucial for determining the speed and nonlinearity of response. Questions remain on whether and when the free electrons are trapped on holes, dopants or defects. The nature of interaction and recombination between the photon-excited species are also important. In this thesis, the crucial early evolution of excited populations is studied with picosecond spectroscopy of optical absorption induced by interband excitation.
subject
Carrier generation & recombination
Defects
Excitons
Scintillators
Transient absorption spectroscopy
Ultrafast pump-probe spectroscopy
contributor
Williams, Richard T (committee chair)
Ghadiri, Elham (committee member)
David, Carroll L (committee member)
Üçer, Kamil Burak (committee member)
Gulthold, Martin (committee member)
date
2019-05-24T08:35:30Z (accessioned)
2020-05-23T08:30:20Z (available)
2019 (issued)
degree
Physics (discipline)
embargo
2020-05-23 (terms)
identifier
http://hdl.handle.net/10339/93909 (uri)
language
en (iso)
publisher
Wake Forest University
type
Dissertation

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