Abstract:
Transition-Metal-doped TiO2 thin films, with nominal composition Ti0.9TM0.1O2-δ (TM ≤ Mn, Fe, Co, Ni, Cu), were grown by pulsed laser deposition (PLD), in order to study the role of dopants in the origin and significance of room temperature ferromagnetism in these systems. The crystallographic structures and their magnetic properties were characterized and the experimental results are compared to ab-initio calculations previously reported. The films are ferromagnetic at room temperature in the cases of Fe, Co, Ni and even Cu impurities, but not in the case of Mn doping. Our results support the hypothesis that oxygen vacancies play a key role in the origin of magnetism in doped TiO2 films, and can explain the diversity of magnetic moments observed experimentally for films grown under different conditions. © 2007 IOP Publishing Ltd.
Registro:
Documento: |
Artículo
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Título: | Ferromagnetism in doped TiO2 thin films prepared by PLD |
Autor: | Duhalde, S.; Rodríguez Torres, C.E.; Vignolo, M.F.; Golmar, F.; Chillote, C.; Cabrera, A.F.; Sánchez, F.H. |
Filiación: | Laboratorio de Ablación Láser, Facultad de Ingeniería, Universidad de Buenos Aires, Paseo Colón 850, 1063 Buenos Aires, Argentina Dpto de Física-IFLP, Fac. Cs. Exactas, Universidad Nacional de la Plata, CC 67, 1900 La Plata, Argentina Laboratorio de Bajas Temperaturas, Fac. de Ciencias Exactas, Universidad de Buenos Aires, Av. Int. Güiraldes 2160, 1428 Buenos Aires, Argentina
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Año: | 2007
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Volumen: | 59
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Número: | 1
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Página de inicio: | 479
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Página de fin: | 482
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DOI: |
http://dx.doi.org/10.1088/1742-6596/59/1/103 |
Título revista: | Journal of Physics: Conference Series
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Título revista abreviado: | J. Phys. Conf. Ser.
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ISSN: | 17426588
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Registro: | https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_17426588_v59_n1_p479_Duhalde |
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Citas:
---------- APA ----------
Duhalde, S., Rodríguez Torres, C.E., Vignolo, M.F., Golmar, F., Chillote, C., Cabrera, A.F. & Sánchez, F.H.
(2007)
. Ferromagnetism in doped TiO2 thin films prepared by PLD. Journal of Physics: Conference Series, 59(1), 479-482.
http://dx.doi.org/10.1088/1742-6596/59/1/103---------- CHICAGO ----------
Duhalde, S., Rodríguez Torres, C.E., Vignolo, M.F., Golmar, F., Chillote, C., Cabrera, A.F., et al.
"Ferromagnetism in doped TiO2 thin films prepared by PLD"
. Journal of Physics: Conference Series 59, no. 1
(2007) : 479-482.
http://dx.doi.org/10.1088/1742-6596/59/1/103---------- MLA ----------
Duhalde, S., Rodríguez Torres, C.E., Vignolo, M.F., Golmar, F., Chillote, C., Cabrera, A.F., et al.
"Ferromagnetism in doped TiO2 thin films prepared by PLD"
. Journal of Physics: Conference Series, vol. 59, no. 1, 2007, pp. 479-482.
http://dx.doi.org/10.1088/1742-6596/59/1/103---------- VANCOUVER ----------
Duhalde, S., Rodríguez Torres, C.E., Vignolo, M.F., Golmar, F., Chillote, C., Cabrera, A.F., et al. Ferromagnetism in doped TiO2 thin films prepared by PLD. J. Phys. Conf. Ser. 2007;59(1):479-482.
http://dx.doi.org/10.1088/1742-6596/59/1/103