Home > Publications database > Dependence of the adsorption height of graphenelike adsorbates on their dimensionality |
Journal Article | FZJ-2018-04249 |
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2018
Inst.
Woodbury, NY
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Please use a persistent id in citations: http://hdl.handle.net/2128/19628 doi:10.1103/PhysRevB.98.075410
Abstract: Comparing the adsorption heights of various graphene nanoribbons on Cu(111) and Au(111) surfaces to those of graphene and π-conjugated planar organic molecules, we observe that two-dimensional graphene adsorbs much further away from the surface than both one-dimensional graphene nanoribbons and π-conjugated planar molecules -- which represent zero-dimensional graphene flakes. We show that this is a direct consequence of the adsorbates' dimensionality. Our results provide invaluable insights into the interplay of Pauli repulsion, pushback effect and chemical interaction for graphene-like adsorbates of any dimensionality on metal surfaces.
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