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Accelerating simulations using REDCHEM_v0.0 for atmospheric chemistry mechanism reduction

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Lelieveld,  Jos
Atmospheric Chemistry, Max Planck Institute for Chemistry, Max Planck Society;

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Citation

Nikolaou, Z. M., Chen, J.-Y., Proestos, Y., Lelieveld, J., & Sander, R. (2018). Accelerating simulations using REDCHEM_v0.0 for atmospheric chemistry mechanism reduction. Geoscientific Model Development, 11(8), 3391-3407. doi:10.5194/gmd-11-3391-2018.


Cite as: https://hdl.handle.net/21.11116/0000-0003-0635-B
Abstract
Chemical mechanism reduction is common practice in combustion research for accelerating numerical simulations; however, there have been limited applications of this practice in atmospheric chemistry. In this study, we employ a powerful reduction method in order to produce a skeletal mechanism of an atmospheric chemistry code that is commonly used in air quality and climate modelling. The skeletal mechanism is developed using input data from a model scenario. Its performance is then evaluated both a priori against the model scenario results and a posteriori by implementing the skeletal mechanism in a chemistry transport model, namely the Weather Research and Forecasting code with Chemistry. Preliminary results, indicate a substantial increase in computational speed-up for both cases, with a minimal loss of accuracy with regards to the simulated spatio-temporal mixing ratio of the target species, which was selected to be ozone.