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要旨

We show that absorption spectra of aluminum chloride phthalocyanine (AlClPc) in the liquid phase can be dynamically modified through the time-resolved interaction with a second laser pulse during a time window on the order of 100 fs. The observed effects can be explained by laser-induced coherent coupling dynamics between the ground state and a bath of excited states as reproduced by a few-level toy model. The presented results help to understand how intense laser fields interact with complex molecules in solution, but in their laser-controlled response still much alike isolated atoms in the gas phase. This understanding can, in the future, be used to modify and control the dynamics in complex systems.