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Journal Article

Self-Organized Chemical Nanoscale Microreactors

MPS-Authors
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Hildebrand,  Michael
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Mikhailov,  Alexander S.
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Ertl,  Gerhard
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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PhysRevLett.83.1475.pdf
(Publisher version), 126KB

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Citation

Hildebrand, M., Kuperman, M., Wio, H., Mikhailov, A. S., & Ertl, G. (1999). Self-Organized Chemical Nanoscale Microreactors. Physical Review Letters, 83(7), 1475-1478. doi:10.1103/PhysRevLett.83.1475.


Cite as: https://hdl.handle.net/21.11116/0000-0008-DD60-3
Abstract
Nonequilibrium localized structures of submicrometer and nanometer sizes, carrying the reaction, can spontaneously develop under reaction conditions on a catalytic surface. These self-organized microreactors emerge because of the coupling between the reaction and a structural phase transition in the substrate. The corresponding localized solutions are constructed using the singular perturbation approximation and reproduced in numerical simulations.