Mn (II) sub-nanometric sites stabilization in noble, N-doped carbonaceous 
materials for electrochemical CO2 reduction

Kossmann, Janina; Ortíz Sánchez-Manjavacas, María Luz; Brandt, Jessica; Heil, Tobias; Lopez Salas, Nieves; Albero , Josep

doi:10.1039/D2CC00585A

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Mn (II) sub-nanometric sites stabilization in noble, N-doped carbonaceous materials for electrochemical CO₂ reduction

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/persons/resource/persons251960

Kossmann, Janina
Nieves Lopez Salas, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

Ortíz Sánchez-Manjavacas, María Luz
Nieves Lopez Salas, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons121167

Brandt, Jessica
Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons206227

Heil, Tobias
Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

/persons/resource/persons228884

Lopez Salas, Nieves
Nieves Lopez Salas, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

Albero , Josep
Nieves Lopez Salas, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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引用

Kossmann, J., Ortíz Sánchez-Manjavacas, M. L., Brandt, J., Heil, T., Lopez Salas, N., & Albero, J. (2022). Mn (II) sub-nanometric sites stabilization in noble, N-doped carbonaceous materials for electrochemical CO₂ reduction. Chemical Communications, 58(31), 4841-4844. doi:10.1039/D2CC00585A.

引用: https://hdl.handle.net/21.11116/0000-000A-2BE0-9

要旨

The preparation of stable and efficient electrocatalysts comprising abundant and non-critical row-materials is of paramount importance for its industrial implementation. Herein, we present a simple synthetic route to prepare Mn(II) sub-nanometric active sites over a highly N-doped noble carbonaceous support. This support not only promotes a strong stabilization of the Mn (II) sites, improving its stability against oxidation, but also provides a convenient coordination environment in the Mn (II) sites able to produce CO, HCOOH and CH3COOH from the electrochemically CO2 reduction.