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| Título: | Supporting Information for: Nonlinear optical response of a plasmonic nanoantenna to circularly polarized light: Rotation of multipolar charge density and near-field spin angular momentum inversion |
Autor: | Quijada, Marina; Babaze, Antton CSIC ORCID; Aizpurua, Javier CSIC ORCID ; Borisov, Andrei G. CSIC | Fecha de publicación: | 2023 | Editor: | American Chemical Society | Citación: | Quijada, Marina; Babaze, Antton; Aizpurua, Javier; Borisov, Andrei G.; 2023; Supporting Information for: Nonlinear optical response of a plasmonic nanoantenna to circularly polarized light: Rotation of multipolar charge density and near-field spin angular momentum inversion [Dataset]; American Chemical Society; https://doi.org/10.1021/acsphotonics.3c00783 | Descripción: | Expression for the circularly polarized fundamental field convenient for an analysis of nonlinear effects; definition of the charge multipoles in cylindrical coordinates and induced potential of the nanowire; analysis of the induced nonlinear near field; definition of the linear multipolar polarizabilities; discussion on the time-to-frequency Fourier transform used to analyze the time-dependent results of the TDDFT and to obtain the frequency-resolved quantities; classical nonretarded calculations of the linear response; extended discussion of the symmetry constraints for the bulk contribution to nonlinear polarization; derivation of the selection rules based on the nonlinear density response formalism; results showing magnetization of the nanowire by a circularly polarized fundamental field pulse; and discussion of the Friedel oscillations of the ground-state electron density (PDF). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at the fundamental frequency (n = 1) for circular polarization with SAM = 1 of the incoming field (MP4). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at the n = 2 harmonic for circular polarization with SAM = 1 of the incoming field (MP4). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at the n = 3 harmonic for circular polarization with SAM = 1 of the incoming field (MP4). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at n = 4 harmonic for circular polarization with SAM = 1 of the incoming field (MP4). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at the fundamental frequency (n = 1) for linear polarization of the incoming field (MP4). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at the n = 2 harmonic for linear polarization of the incoming field (MP4). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at the n = 3 harmonic for linear polarization of the incoming field (MP4). Time evolution of the charge density induced in the nanowire, δϱ(n)(r, t) = Re{δϱ(r, nΩ)e–inΩt }, at the n = 4 harmonic for linear polarization of the incoming field (MP4). | URI: | http://hdl.handle.net/10261/342602 | DOI: | 10.1021/acsphotonics.3c00783 | Referencias: | Quijada, Marina; Babaze, Antton; Aizpurua, Javier; Borisov, Andrei G.. Nonlinear optical response of a plasmonic nanoantenna to circularly polarized light: Rotation of multipolar charge density and near-field spin angular momentum inversion. https://doi.org/10.1021/acsphotonics.3c00783. http://hdl.handle.net/10261/342600 |
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