Comment on "engineering coherence among excited states in synthetic heterodimer 
systems"

Halpin, A.; Johnson, P. J. M.; Miller, R. J. D.

doi:10.1126/science.1250926

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Comment on "engineering coherence among excited states in synthetic heterodimer systems"

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Miller, R. J. D.
Institute for Optical Sciences, Departments of Chemistry and Physics, University of Toronto, 80 Saint George Street, Toronto, ON M5S 3H6, Canada;
Miller Group, Atomically Resolved Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

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https://dx.doi.org/10.1126/science.1250926
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Zitation

Halpin, A., Johnson, P. J. M., & Miller, R. J. D. (2014). Comment on "engineering coherence among excited states in synthetic heterodimer systems". Science, 344(6188), 1099-b-1099-b. doi:10.1126/science.1250926.

Zitierlink: https://hdl.handle.net/11858/00-001M-0000-0024-BE15-C

Zusammenfassung

Hayes et al. (Reports, 21 June 2013, p. 1431) used two-dimensional (2D) electronic spectroscopy to study molecular heterodimers and reported a general mechanism for the prolongation of electronic coherences, consistent with previous interpretations of 2D spectra for light-harvesting systems. We argue that the dynamics attributed to electronic coherences are inconclusive based on experimental inconsistencies arising from limited sample characterization and insufficient control measurements.