Observation of Floquet states in graphene

Merboldt, M.; Schüler, M.; Schmitt, D.; Bange, J. P.; Bennecke, W.; Gadge, K.; Pierz, K.; Schumacher, H. W.; Momeni, D.; Steil, D.; Manmana, S. R.; Sentef, M. A.; Reutzel, M.; Mathias, S.

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Observation of Floquet states in graphene

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Sentef, M. A.
Institute for Theoretical Physics and Bremen Center for Computational Materials Science, University of Bremen;
Theoretical Description of Pump-Probe Spectroscopies in Solids, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;
Center for Free-Electron Laser Science (CFEL);

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https://arxiv.org/abs/2404.12791
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2404.12791.pdf
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Citation

Merboldt, M., Schüler, M., Schmitt, D., Bange, J. P., Bennecke, W., Gadge, K., et al. (2024). Observation of Floquet states in graphene.

Cite as: https://hdl.handle.net/21.11116/0000-000F-30C5-C

Abstract

Recent advances in the field of condensed-matter physics have unlocked the potential to realize and control emergent material phases that do not exist in thermal equilibrium. One of the most promising concepts in this regard is Floquet engineering, the coherent dressing of matter via time-periodic perturbations. However, the broad applicability of Floquet engineering to quantum materials is still unclear. For the paradigmatic case of monolayer graphene, the theoretically predicted Floquet-induced effects, despite a seminal report of the light-induced anomalous Hall effect, have been put into question. Here, we overcome this problem by using electronic structure measurements to provide direct experimental evidence of Floquet engineering in graphene. We report light-matter-dressed Dirac bands by measuring the contribution of Floquet sidebands, Volkov sidebands, and their quantum path interference to graphene's photoemission spectral function. Our results finally demonstrate that Floquet engineering in graphene is possible, paving the way for the experimental realization of the many theoretical proposals on Floquet-engineered band structures and topological phases.